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Realcat

Production scientifique

Chapitre de livre

1 - Biorefinery: From Biomass to Chemicals and Fuels

Editors: M. Artesta, A. Dibenedetto, F. Dumeignil

15 Hybrid catalysis: bridging two worlds for greener chemicals and energy production, pages 493-536

E. Heuson and A. Dibenedetto

DOI: 10.1515/9783110705386-016


2 - Modern Applications of High Throughput R&D in Heterogeneous Catalysis

Editors: A. Hagemeyer, A. F. Volpe

Chapter 9.3, A Novel Integrated High-Throughput Approach for Catalytic Reactions Development: The REALCAT Concept, p. 324-337

F. Dumeignil, L. Montagne, R. Froidevaux, S. Heyte, S. Paul

eISBN: 978-1-60805-872-3

ISBN: 978-1-60805-873-0

Bentham e-books (2014)

DOI: 10.2174/97816080587231140101


Articles

1 - Hybrid monometallic and bimetallic copper-palladium zeolite catalysts for direct synthesis of dimethyl ether from CO2

S. Navarro-Jaén, M. Virginie, J. Thuriot-Roukos, R. Wojcieszak, A. Khodakov

New J. Chem. (2022-01)

DOI: 10.1039/D1NJ05734K


2 - Structure-performance correlations in the hybrid oxide-supported copper-zinc SAPO-34 catalysts for direct synthesis of dimethyl ether from CO2

S. Navarro-Jaén, M. Virginie, J. Thuriot-Roukos, R. Wojcieszak, A. Khodakov

J. Mater. Sci. (2022-01)

DOI: 10.1007/s10853-022-06890-w


3 - Heterogenization of Complexes by Encapsulation in Solid Micelles for Aqueous-Phase Catalysis.

Q. Wang, W-J. Zhou, S. Heyte, J. Thuriot-Roukos, M. Marinova, A. Addad, S. Rouzière, P. Simon, M. Capron and V. V. Ordomsky

Chem. Mater. (2022-01)

DOI: 10.1021/acs.chemmater.1c02741


4 - Versatility of supported gold nanoparticles on hydrotalcites used for oxidation and reduction reactions

F. Drault, Y. Snoussi, C. P. Ferraz, J. Thuriot-Roukos, S. Heyte, I. Itabaiana Junior, M. Marinova, S. Paul and R. Wojcieszak

Catalysis Research (2022-01)

DOI: 10.21926/cr.2201001


5 - Selective aqueous phase hydrogenation of xylose to xylitol over SiO2-supported Ni and Ni-Fe catalysts: Benefits of promotion by Fe

A. Sadier, D. Shi, A.-S. Mamede, S. Paul, E. Marceau and R. Wojcieszak

Appl. Catal. B : Env. (2021-12)

DOI: 10.1016/j.apcatb.2021.120564


6 - Influence of Pd and Pt promotion in Gold based bimetallic catalysts on selectivity modulation in Furfural? base-free oxidation

H. K. Al Rawas, C. P. Ferraz, J. Thuriot-Roukos, S. Heyte, S. Paul and R. Wojcieszak

Catalysts (2021-10)

DOI: 10.3390/catal11101226


7 - Ru(III) single site solid micellar catalyst for selective aqueous phase hydrogenation of carbonyl groups in biomass-derived compounds

Q. Wang, S. Santos, C. A. Urbina-Blanco, W. Zhou, Y. Yang, M. Marinova, S. Heyte, J. Thuriot-Roukos, O. Ersen, W. Baaziz, O. V. Safonova, M. Saeys and V. V. Ordomsky

Applied Catalysis B: Environmental (2021-09)

DOI: 10.1016/j.apcatb.2021.120730


8 - Investigating the active phase of Ca-based glycerol polymerization catalysts: On the importance of calcium glycerolate

N. Ebadipour, F. Dumeignil, B. Katryniok, L. Delevoye, B. Revel and S. Paul

Mol. Catal. (2021-05)

DOI: 10.1016/j.mcat.2021.111571


9 - Study of the direct CO2 carboxylation reaction on supported metal nanoparticles

F. Drault, Y. Snoussi, J. Thuriot-Roukos, I. Jr Itabaiana, S. Paul and R. Wojcieszak

Catalysts (2021-03)

DOI: 10.3390/catal11030326


10 - Ruthenium-Catalyzed Coupling Reactions of CO2 with C2H4 and Hydrosilanes towards Silyl Esters

E. Kirillov, K. Kunihiro, S. Heyte, S. Paul, T. Roisnel, J.-F. Carpentier

ChemEurJ. (2021-02)

DOI: 10.1002/chem.202005083


11 - Efficient non-noble Ni-Cu based catalysts for the valorization of palmitic acid through decarboxylation reaction

C. P. Ferraz, A. Kimene, K. Silva, S. Heyte, C. Durlin, O. Simon, F. Dumeignil, S. Paul and R. Wojcieszak

Catal. Sc. Technol. (2021-01)

DOI: 10.1039/D0CY02161J


12 - Hybrid conversion of 5-hydroxymethylfurfural to 5-aminomethyl-2-furancarboxylic acid: toward new bio-sourced polymers

A. Lancien, R. Wojcieszak, E. Cuvelier, M. Duban, P. Dhulster, S. Paul, F. Dumeignil, R. Froidevaux and E. Heuson

ChemCatChem (2020-11)

DOI: 10.1002/cctc.202001446


13 - Plasmon-Driven Electrochemical Methanol Oxidation on Gold Nanohole Electrodes

L. Pang, A. Barras, V. Mishyn, S. Heyte, E. Heuson, H. Oubaha, G. Sandu, S. Melinte, R. Boukherroub and S. Szunerits

ACS Applied Materials & Interfaces (2020-10)

DOI: 10.1021/acsami.0c14436


14 - L’avènement des matériaux multi-catalytiques hybrides, vers une combinaison optimale des catalyseurs

E. Heuson, R. Froidevaux, I. Itabaiana Jr, R. Wojcieszak, C. Capron and F. Dumeignil

L'Actualité Chimique (2020-09)


15 - Cinquante nuances de catalyse hybride

E. Heuson, R. Froidevaux, J.-S. Girardon, I. Itabaiana Jr, R. Wojcieszak, C. Capron and F. Dumeignil

L'Actualité Chimique (2020-09)


16 - Des réactions multi-catalytiques au concept de catalyse hybride

E. Heuson, R. Froidevaux, I. Itabaiana Jr, R. Wojcieszak, C. Capron and F. Dumeignil

L'Actualité Chimique (2020-09)


17 - La catalyse, la diversité au service de l’efficacité

E. Heuson, R. Froidevaux, I. Itabaiana Jr, R. Wojcieszak, C. Capron and F. Dumeignil

L'Actualité Chimique (2020-09)


18 - The Various Levels of Integration of Chemo- and Bio-Catalysis towards Hybrid Catalysis

E. Heuson and F. Dumeignil

Catalysis Science & Technology (2020-08)

DOI: 10.1039/D0CY00696C


19 - Dataset on phenotypic characterization, on protein and genome analysis of three fluorescent Pseudomonas strains from mid-mountain water

E. Dussert, M. Tourret, B. Deracinois, M. Duban, V. Lecle?re, B. Cudennec, R. Ravallec, J. Behra-Miellet

Data in Brief (2020-06)

DOI: 10.1016/j.dib.2020.105466


20 - A Leaderless Two-Peptide Bacteriocin, Enterocin DD14, Is Involved in Its Own Self-Immunity: Evidence and Insights

R. Ladjouzi, A. Lucau-Danila, A. Benachour, D. Drider

Frontiers in Bioengineering and Biotechnology (2020-06)

DOI: 10.3389/fbioe.2020.00644


21 - Lactic acid conversion to acrylic acid over fluoride-substituted hydroxyapatites

R. Wojcieszak, T. Bonnotte, S. Paul, B. Katryniok and F. Dumeignil

Front. Chem. (2020-05)

DOI: 10.3389/fchem.2020.00421


22 - In Vitro Characterisation of the Antioxidative Properties of Whey Protein Hydrolysates Generated under pH- and Non pH-Controlled Conditions

T. Kleekayai, A. V. Le Gouic, B. Deracinois, B. Cudennec and R. J. FitzGerald

Foods (2020-05)

DOI: 10.3390/foods9050582


23 - Raman Spectroscopy applied to monitor Furfural liquid-phase oxidation catalyzed by supported Gold nanoparticles

J. Thuriot-Roukos, R. Khadraoui, S. Paul and R. Wojcieszak

ACS Omega (2020-04)

DOI: 10.1021/acsomega.0c00091


24 - Aerobic oxidation of 1,6-hexanediol to adipic acid over Au-based catalysts: the role of basic support

N. Capece, A. Sadier, C. Ferraz, J. Thuriot-Roukos, M. Pietrowski, M. Zieli?ski, S. Paul F. Cavani and R. Wojcieszak

Catal. Sc. Technol. (2020-03)

DOI: 10.1039/D0CY00183J


25 - Enzymatic depolymerization of industrial lignins by laccase-mediator systems in 1,4-dioxane/water

J. Dillies, C. Vivien, M. Chevalier, A. Rulence, G. Chaitaigne, C. Flahaut, V. Senez, R. Froidevaux

Biotechnology and Applied Biochemistry (2020-03)

DOI: 10.1002/bab.1887


26 - Fluorescent Pseudomonas strains from mid-mountain water able to release antioxidant proteins directly into water

E. Dussert, M. Tourret, B. Deracinois, M. Duban, V. Lecle?re, B. Cudennec, R. Ravallec, J. Behra-Miellet

Microbiological Research (2020-02)

DOI: 10.1016/j.micres.2020.126444


27 - 5-Hydroxymethylfurfural and Furfural Base-Free Oxidation over AuPd Embedded Bimetallic Nanoparticles

C. P. Ferraz, N. J. S. Costa, E. Teixeira-Neto, A. A. Teixeira-Neto, C. W. Liria, J. Thuriot-Roukos, M. Teresa Machini, R. Froidevaux, F. Dumeignil, L. M. Rossi and R. Wojcieszak

Catalysts (2020-01)

DOI: 10.3390/catal10010075


28 - Proteolytic activity of Lactobacillus strains isolated from Mongolian traditional dairy products: A multiparametric analysis

C. Raveschot, B. Cudennec, B. Deracinois, M. Fre?mont, M. Vaeremans, J. Dugersurenc, S. Demberel, D. Drider, P. Dhulster, F. Coutte, C. Flahaut

Food Chemistry (2020-01)

DOI: 10.1016/j.foodchem.2019.125415


29 - High Added-Value Co-Product: the Porcine Cruor is an Attractive Source of Active Peptides

O. Zouari, R. Przybylski, M. Hannioui, L. Sion, P. Dhulster, N. Nedjar-Arroume

Journal of Nutritional Health & Food Science (2020-01)

DOI: 10.15226/jnhfs.2020.001170


30 - Liquid Phase Furfural Oxidation under Uncontrolled pH in Batch and Flow Conditions: The Role of In Situ Formed Base

A. Roselli, Y. Carvalho, F. Dumeignil, F. Cavani, S. Paul, R. Wojcieszak

Catalysts (2020-01)

DOI: 10.3390/catal10010073


31 - 5-Hydroxymethylfurfural and Furfural Base-Free Oxidation over AuPd Embedded Bimetallic Nanoparticles

C. P. Ferraz, N. J. S. Costa, E. Teixeira-Neto, A?. A. Teixeira-Neto, C. W. Liria, J. Thuriot-Roukos, M. Teresa Machini, R. Froidevaux, F. Dumeignil, L. M. Rossi, R. Wojcieszak

Catalysts (2020-01)

DOI: 10.3390/catal10010075


32 - Proteolytic activity of Lactobacillus strains isolated from Mongolian traditional dairy products: A multiparametric analysis

C. Raveschot, B. Cudennec, B. Deracinois, M. Frémont, M. Vaeremans, J. Dugersuren, S. Demberel, D. Drider, P. Dhulster, F. Coutte, C. Flahaut

Food Control (2020-01)

DOI: 10.1016/j.foodchem.2019.125415


33 - Molecular strategies for adapting Bacillus subtilis 168 biosurfactant production to biofilm cultivation mode

H.-L. Brück, F. Delvigne, P. Dhulster, P. Jacques, F. Coutte

Bioresource Technology (2019-12)

DOI: 10.1016/j.biortech.2019.122090


34 - Bio-emulsifying and biodegradation activities of syringafactin producing Pseudomonas spp. strains isolated from oil contaminated soils

O. Zouari, D. Lecouturier, A. Rochex, G. Chataigne, P. Dhulster, P. Jacques, D. Ghribi

Biodegradation (2019-10)

DOI: 10.1007/s10532-018-9861-x


35 - Esterificac?a?o oxidativa de derivados de biomassa com catalisadores de Au suportados em o?xidos ba?sicos

C. P. Ferraz, A. H. Braga, L. M. Rossi, R. Wojcieszak, F. Dumeignil

SBCat (2019-09)


36 - Influence of the structure of trigonal Mo-V-M3rd oxides (M3rd?=?-, Fe, Cu, W) on catalytic performances in selective oxidations of ethane, acrolein, and allyl alcohol

S. Ishikawa, T. Murayama, B. Katryniok, F. Dumeignil, M. Araqued, S. Heyte, S. Paul, Y. Yamada, M. Iwazaki, N. Noda, W. Ueda

Catalysis Today (2019-09)

DOI: 10.1016/j.apcata.2019.117151


37 - Au-based bimetallic catalysts: how the synergy between two metals affects their catalytic activity

J. Sha, S. Paul, F. Dumeignil, R. Wojcieszak

RSC Advances (2019-09)

DOI: 10.1039/c9ra06001d


38 - Fully integrated high-throughput methodology for the study of Ni- and Cusupported catalysts for glucose hydrogenation

S. Silvester, F. Ramos, J. Thuriot-Roukos, S. Heyte, M. Araque, S. Paul, R. Wojcieszak

Catalysis Today (2019-05)

DOI: 10.1016/j.cattod.2019.05.041


39 - Modelling and optimisation of gas-liquid mass transfer in a microporous hollow fiber membrane aerated bioreactor used to produce surfactin

A. Berth, D. Lecouturier, K. Loubiere, P. Dhulster, G. Delaplace

Biochemical Engineering Journal (2019-05)

DOI: 10.1016/j.bej.2018.10.029


40 - Horseradish peroxidase-AuNP/LDH heterostructures: influence on nanogold release and enzyme activity

E.-F. Grosu, R. Froidevaux, G. Carja

Gold Bulletin (2019-04)

DOI: 10.1007/s13404-019-00256-y


41 - Innovative microscale workflow from fungi cultures to Cell Wall-Degrading Enzyme screening

R. Raulo, E. Heuson, A. Siah, V. Phalip and R. Froidevaux

Microbial Biotechnology (2019-03)

DOI: 10.1111/1751-7915.13405


42 - Direct amination of 1-octanol with NH3 over Ag-Co/Al2O3: Promoting effect of the H2 pressure on the reaction rate

J. Ibañez, M. Araque-Marin, S. Paul, M. Pera-Titus

Chemical Engineering Journal (2019-02)

DOI: 10.1016/j.cej.2018.10.021


43 - Exploiting the Synergetic Behavior of PtPd Bimetallic Catalysts in the Selective Hydrogenation of Glucose and Furfural

P. M. de Souza, L. Silvester, A. G. M. da Silva, C. G. Fernandes, T. S. Rodrigues, S. Paul, P. C. Camargo, R. Wojcieszak

Catalysts (2019-02)

DOI: 10.3390/catal9020132


44 - Cyclodextrin-assisted low-metal Ni-Pd/Al2O3 bimetallic catalysts for the direct amination of aliphatic alcohols

A. Tomer, B.T. Kusema, J.-F. Paul, C. Przybylski, E. Monflier, M. Pera-Titus, A. Ponchel

Journal of Catalysis (2018-12)

DOI: 10.1016/j.jcat.2018.10.002


45 - Bimetallic Fe-Ni/SiO2 catalysts for furfural hydrogenation: Identification of the interplay between Fe and Ni during deposition-precipitation and thermal treatments

D. Shi, Q. Yang, C. Peterson, A.-F. Lamic-Humblot, J.-S. Girardon, A. Constant-Griboval, L. Stievano, M. T. Sougrati, V. Briois, P. A. J. Bagot, R. Wojcieszak, S. Paul, E. Marceau

Catalysis Today (2018-11)

DOI: 10.1016/j.cattod.2018.11.041


46 - Design of a multi-well plate for high-throughput characterization of heterogeneous catalysts by XRD, FT-IR, Raman and XRF spectroscopies

J. Thuriot-Roukos, M. Bennis, E. Heuson, P. Roussel, F. Dumeignil, S. Paul

RSC Advances (2018-11)

DOI: 10.1039/c8ra08216b


47 - Screening of Lipopeptide-Producing Strains of Bacillus sp. Using a New Automated and Sensitive Fluorescence Detection Method

E. Heuson, A. Etchegaray, S. L. Filipe, D. Beretta, M. Chevalier, V. Phalip, and F. Coutte

Biotechnology Journal (2018-11)

DOI: 10.1002/biot.201800314


48 - Combining Active Phase and Support Optimization in MnO2-Au Nanoflowers: Enabling High Activities Toward Green Oxidations

A. da Silva, T. Rodrigues, E. Candido, I. de Freitas, A. da Silva, H. Fajardo, R. Balzer, J. Gomes, J. Assaf, D. de Oliveira, N. Oger, S. Paul, R. Wojcieszak, P. H. C. Camargo

Journal of Colloid and Interface Science (2018-11)

DOI: 10.1016/j.jcis.2018.06.089


49 - From sequential chemoenzymatic synthesis to integrated hybrid catalysis: taking the best of both worlds to open up the scope of possibilities for a sustainable future

F. Dumeignil, M. Guehl, A. Gimbernat, M. Capron, N. Lopes Ferreira, R.
Froidevaux, J.-S. Girardon, R. Wojcieszak, P. Dhulster, D. Delcroix

Catalysis Science & Technology (2018-09)

DOI: 10.1039/C8CY01190G


50 - Ruthenium silica nanoreactors with varied metal–wall distance for efficient control of hydrocarbon distribution in Fischer–Tropsch synthesis

Y. Chen, N. Batalha, M. Marinova, M. Impéror-Clerc, C. Ma, O. Ersen, W. Baaziz, J.A. Stewart, D. Curulla-Ferré, A.Y. Khodakov, V.V. Ordomsky

Journal of Catalysis (2018-09)

DOI: 10.1016/j.jcat.2018.06.023


51 - Influence of Support Basic Sites in Green Oxidation of Biobased Substrates Using Au-Promoted Catalysts

C.P. Ferraz, M. Zieli?ski, M. Pietrowski, S. Heyte, F. Dumeignil, L.M. Rossi, R. Wojcieszak

ACS Sustainable Chemistry & Engineering (2018-09)

DOI: 10.1021/acssuschemeng.8b03330


52 - Development of horseradish peroxidase/layered double hydroxide hybrid catalysis for phenol degradation

E.-F. Grosu, G. Carja, R. Froidevaux

Research on Chemical Intermediates (2018-08)

DOI: 10.1007/s11164-018-3583-x


53 - From a Sequential Chemo-Enzymatic Approach to a Continuous Process for HMF Production from Glucose

A. Gimbernat, M. Guehl, N. L. Ferreira, E. Heuson, P. Dhulster, M. Capron, F. Dumeignil, D. Delcroix, J.-S. Girardon and R. Froidevaux

Catalysts (2018-08)

DOI: 10.3390/catal8080335


54 - High-throughput optimization of medium components and culture conditions for the efficient production of a lipopeptide pseudofactin by Pseudomonas fluorescens BD5

P. Biniarz, F. Coutte, F. Gancel and M. Lukaszewicz

Microbial Cell Factories (2018-08)

DOI: 10.1186/s12934-018-0968-x


55 - Furfural oxidation on gold supported on MnO2 oxides: Influence of the support structure on the catalytic performances

C. Ferraz, A. G. M. Da Silva, T. S. Rodrigues, S. Paul, P. Camargo, R. Wojcieszak

Applied Sciences (2018-07)

DOI: 10.3390/app8081246


56 - Cyclohexane oxidation to adipic acid under green conditions: a scalable and sustainable process

A. Mazzi, S. Paul, F. Cavani, R. Wojcieszak

ChemCatChem (2018-06)

DOI: 10.1002/cctc.201800419


57 - Formation of peptide layers and adsorption mechanisms on a negatively charged cation-exchange membrane

M. Persico, S. Mikhaylin, A. Doyen, L. Firdaous, R. Hammami, M. Chevalier, C. Flahaut, P. Dhulster, L. Bazinet

Journal of Colloid and Interface Science (2017-12)

DOI: 10.1016/j.jcis.2017.08.029


58 - Mixed oxides supported low-nickel formulations for the direct amination of aliphatic alcohols with ammonia

A. Tomer, Z. Yan, A. Ponchel, M. Pera-Titus

Journal of Catalysis (2017-12)

DOI: 10.1016/j.jcat.2017.08.015


59 - Facile preparation of Ni/Al2O3 catalytic formulations with the aid of cyclodextrin complexes: Towards highly active and robust catalysts for the direct amination of alcohols

A Tomer, F. Wyrwalski, C. Przybylski, J-F. Paul, E. Monflier, M. Pera-Titus, A. Ponchel

Journal of Catalysis (2017-12)

DOI: 10.1016/j.jcat.2017.10.006


60 - Isolation and Characterization of Bacteria Colonizing Acartia tonsa Copepod Eggs and Displaying Antagonist Effects against Vibrio anguillarum, Vibrio alginolyticus and Other Pathogenic Strains

M. Zidour, M. Chevalier, Y. Belguesmia, B. Cudennec, T. Grard, D. Drider, S. Souissi and C. Flahaut

Frontiers in Microbiology (2017-10)

DOI: 10.3389/fmicb.2017.01919


61 - Design of nanocomposites with cobalt encapsulated in the zeolite micropores for selective synthesis of isoparaffins in Fischer–Tropsch reaction

A. Carvalho, M. Marinova, N. Batalha, N. R. Marcilio, A. Y. Khodakov and V. V. Ordomsky

Catalysis Science & Technology (2017-10)

DOI: 10.1039/c7cy01945a


62 - Polyoxometalate, Cationic Cluster, and ??Cyclodextrin: From Primary Interactions to Supramolecular Hybrid Materials

M. Moussawi, N. Leclerc-Laronze, S. Floquet, P. Abramov, M. Sokolov, S. Cordier, A. Ponchel, E. Monflier, H. Bricout, D. Landy, M. Haouas, J. Marrot and E. Cadot

Journal of the American Chemical Society (2017-08)

DOI: 10.1021/jacs.7b07317


63 - Interactions between Kluyveromyces marxianus from cheese origin and the intestinal symbiont Bacteroides thetaiotaomicron: Impressive antioxidative effects

A. Ceugniez, M. Tourret, E. Dussert, F. Coucheney,B. Deracinois, P. Jacques, C. Flahaut, E. Heuson, D. Drider, J. Behra-Miellet

LWT - Food Science and Technology (2017-08)

DOI: 10.1016/j.lwt.2017.03.056


64 - Soldering of Iron Catalysts for Direct Synthesis of Light Olefins from Syngas under Mild Reaction Conditions

V. V. Ordomsky, Y. Luo, B. Gu, A. Carvalho, P. A. Chernavskii, K. Cheng, and A. Y. Khodakov

ACS Catalysis (2017-08)

DOI: 10.1021/acscatal.7b01307


65 - REALCAT : une plateforme unique au monde dédiée au développement haut débit de catalyseurs pour les bioraffineries

S. Paul, F. Dumeignil

L’Actualité Chimique (2017-07)


66 - Genetic engineering of the branched fatty acid metabolic pathway of Bacillus subtilis for the overproduction of surfactin C14 isoform

D. Dhali, F. Coutte, A. Argüelles Arias, S. Auger, V. Bidnenko, G; Chataigné, M. Lalk, J. Niehren, J. de Sousa, C. Versari and P. Jacques

Biotechnology Journal (2017-07)

DOI: 10.1002/biot.201600574


67 - Heterogeneous catalysis with renewed attention: principles, theories and concepts

F. Dumeignil, J.-F. Paul, S. Paul

Journal of Chemical Education (2017-03)

DOI: 10.1021/acs.jchemed.6b00611


68 - The safe enterocin DD14 is a leaderless two-peptide bacteriocin with anti-Clostridium perfringens activity

D. L. Caly, M. Chevalier, C. Flahaut, B. Cudennec, A. Khassaf Al Atya, G. Chataigné, R. D’Inca, E. Auclair, D. Drider

International Journal of Antimicrobial Agents (2017-03)

DOI: 10.1016/j.ijantimicag.2016.11.016


69 - Syngas to Chemicals: The Incorporation of Aldehydes into Fischer–Tropsch Synthesis

V. V. Ordomsky and A. Y. Khodakov

ChemCatChem (2017-03)

DOI: 10.1002/cctc.201601508


70 - High-throughput strategies for the discovery and engineering of enzymes for biocatalysis

P. Jacques, M. Bechet, M. Bigan, D. Caly, G. Chataigne, F. Coutte, C. Flahaut, E. Heuson, V. Leclere, D. Lecouturier, V. Phalip, R. Ravallec, P. Dhulster, R. Froidevaux

Bioprocess Biosyst Engineering (2017-03)

DOI: 10.1007/s00449-016-1690-x


71 - Oxidation of but-3-en-1,2-diol: Green access to hydroxymethionine intermediate

F. Grasset, P. Rey, V. Bellière-Baca, M. Araque, S. Paul, F. Dumeignil, R. Wojcieszak, B. Katryniok

Catalysis Today (2017-01)

DOI: 10.1016/j.cattod.2016.06.036


72 - Al-doped SBA-15 Catalysts for Low-temperature Dehydration of 1,3-Butanediol into Butadiene

F. Jing, B. Katryniok, S. Paul, L. Fang, A. Liebens, M. Shen, B. Hu, F. Dumeignil, and M. Pera-Titus

ChemCatChem (2017-01)

DOI: 10.1002/cctc.201601202


73 - Effects of co-feeding with nitrogen-containing compounds on the performance of supported cobalt and iron catalysts for Fischer-Tropsch synthesis

V. V. Ordomsky, A. Carvalho, B. Legras, S. Paul, M. Virginie, V. Sushkevich, A. Y. Khodakov

Catalysis Today (2016-10)

DOI: 10.1016/j.cattod.2015.12.015


74 - An improvement of surfactin production by B. subtilis BBG131 using design of experiments in microbioreactors and continuous process in bubbleless membrane bioreactor

L. F. Motta Dos Santos, F. Coutte, R. Ravallec, P. Dhulster, L. Tournier-Couturier, P. Jacques

Bioresource Technology (2016-10)

DOI: 10.1016/j.biortech.2016.07.053


75 - Selective oxidation of glucose to glucuronic acid by cesium-promoted gold nanoparticle catalyst

R. Wojcieszak, I.M. Cuccovia, M.A. Silva, L.M. Rossi

Journal of Molecular Catalysis A: Chemical (2016-10)

DOI: 10.1016/j.molcata.2016.02.008


76 - Role of crystalline structure in allyl alcohol selective oxidation over Mo3VOx complex metal oxide catalysts

T. Murayama, S. Heyte, B. Katryniok, M. Araque, S. Ishikawa, F. Dumeignil, S. Paul, W. Ueda

ChemCatChem (2016-07)

DOI: 10.1002/cctc.201600430


77 - Influence of promoters on the production of fengycin in Bacillus spp.

Y. Yaseen, F. Gancel, D. Drider, M. Bechet, P. Jacques

Research in Microbiology (2016-05)

DOI: 10.1016/j.resmic.2016.01.008


78 - The role of carbon pre-coating for the synthesis of highly efficient cobalt catalysts for Fischer–Tropsch synthesis

K. Cheng, V. Subramanian, A. Carvalho, V. V. Ordomsky, Y. Wang, A. Y. Khodakov

Journal of Catalysis (2016-05)

DOI: 10.1016/j.jcat.2016.02.019


79 - MALDI-TOF mass spectrometry for the identification of lactic acid bacteria isolated from a French cheese: The Maroilles

M. Nacef, M. Chevalier, S. Chollet, D. Drider, C. Flahaut

International Journal of Food Microbiology (2016-04)

DOI: 10.1016/j.ijfoodmicro.2016.07.005


80 - First catalytic asymmetric hydrogenation of quinoxaline-2-carboxylates

A. M. Maj, S. Heyte, M. Araque, F. Dumeignil, S. Paul, I. Suisse, F. Agbossou-Niedercorn

Tetrahedron (2016-03)

DOI: 10.1016/j.tet.2016.01.033


81 - Design of iron catalysts supported on carbonsilica composites with enhanced catalytic performance in high-temperature FischerTropsch synthesis

V. Subramanian, V. Ordomsky, B. Legras, K. Cheng, C. Cordier, P. Chernavskii, A. Khodakov

Catalysis Science & Technology (2016-02)

DOI: 10.1039/c6cy00060f


82 - Direct dehydration of 1,3-butanediol into butadiene over aluminosilicate catalysts

F. Jing, B. Katryniok, M. Araque, R. Wojcieszak, M. Capron, S. Paul, M. Daturi, J.-M. Clacens, F. De Campo, A. Liebens, F. Dumeignil, M. Pera-Titus

Catalysis Science & Technology (2016-02)

DOI: 10.1039/c5cy02211h


83 - Nanoreactors: An efficient tool to control the chain-length distribution in Fischer-Tropsch synthesis

V. Subramanian, K. Cheng, C. Lancelot, S. Heyte, S. Paul, V. V. Ordomsky, A. Y. Khodakov

ACS Catalysis (2016-02)

DOI: 10.1021/acscatal.5b01596


84 - The Role of Steric Effects and Acidity in the Direct Synthesis of iso-Paraffins from Syngas on Cobalt Zeolite Catalysts

V. Subramanian, V. L. Zholobenko, K. Cheng, C. Lancelot, S. Heyte, J. Thuriot, S. Paul, V. V. Ordomsky, A. Y. Khodakov

ChemCatChem (2015-11)

DOI: 10.1002/cctc.201500777


85 - Pore Size Effects in High Temperature Fischer-Tropsch Synthesis over Supported Iron Catalysts

K. Cheng, M. Virginie, V. V. Ordomsky, C. Cordier, P. A. Chernavsky, M. I. Ivantsov, S. Paul, Y. Wang, A. Y. Khodakov

Journal of Catalysis (2015-08)

DOI: 10.1016/j.jcat.2014.12.007


86 - Modeling leucine's metabolic pathway and knockout prediction improving the production of surfactin, a biosurfactant from Bacillus subtilis

F. Coutte, J. Niehren, D. Dhali, M. John, C. Versari, P. Jacques

Biotechnology Journal (2015-08)

DOI: 10.1002/biot.201400541


87 - Sodium-promoted iron catalysts prepared on different supports for high temperature Fischer–Tropsch synthesis

K. Cheng, V. V. Ordomsky, B. Legras, M. Virginie, S. Paul, Y. Wang, A. Y. Khodakov

Applied Catalysis A: General (2015-08)

DOI: 10.1016/j.apcata.2015.06.010


88 - Realcat: a new platform to bring catalysis to the lightspeed

S. Paul, S. Heyte, B. Katryniok, C. Garcia-Sancho, P. Maireles-Torres, F. Dumeignil

Oil & Gas Science and Technology - Revue d'IFP Energies Nouvelle (2015-02)

DOI: 10.2516/ogst/2014052


89 - The role of carbon atoms of supported iron carbides in Fischer-Tropsch synthesis

V. V. Ordomsky, B. Legras, K. Cheng, S. Paul, A. Y. Khodakov

Catalysis Science & Technology (2015-01)

DOI: 10.1039/C4CY01631A


90 - Biomass-derived Platform Molecules Upgrading through Catalytic Processes: Yielding Chemicals and Fuels

F. Dumeignil, M. Capron, B. Katryniok, R. Wojcieszak, A. Lofberg, J-S. Girardon, S.Desset, M. Araque-Marin, L. Jalowiecki-Duhamel, S. Paul

Journal of the Japan Petroleum Institute (2015)

DOI: 10.1627/jpi.58.257


91 - Support effects in high temperature Fischer-Tropsch synthesis on iron catalysts

K. Cheng, V. V. Ordomsky, M. Virginie, B. Legras, P. A. Chernavskii, V. O. Kazak, C. Cordier, S. Paul, Y. Wang, A. Y. Khodakov

Applied Catalysis A: General (2014-11)

DOI: 10.1016/j.apcata.2014.09.033


92 - Cobalt and iron species in alumina supported bimetallic catalysts for Fischer-Tropsch reaction

A. Griboval-Constant, A. Butel, V. V. Ordomsky, P. A. Chernavskii, A. Y. Khodakov

Applied Catalysis 1: General (2014-07)

DOI: 10.1016/j.apcata.2014.04.047


Séminaires invités

1 - Catalytic Processes Development for Biomass Valorisation Using Advanced High-Throughput Technologies

S. Paul, S. Heyte, J. Thuriot-Roukos, A. Kiméné, R. Wojcieszak, F. Dumeignil

10th ICEC & 3rd EECAT, 22-26/09, Tianjin, China (2018)


2 - Innovative high-throughput microplate approach for cell wall degrading enzyme production based on fungi and lignocellulosic raw biomass interaction

E. Heuson, Roxane Raulo, A. Siah, F. Krier, P. Halama, P. Reignault, V. Phalip, R. Froidevaux

Beckman User Meeting, 13-14/06, Berlin, Germany (2018)


3 - The REALCAT platform: high-throughput screening equipment dedicated to biomass valorization

E. Zeyer, B. Cudennec, C. Le Bris, T. Grard, C. Flahaut, B. Deracinois, P. Dhulster, R. Froidevaux, J. Thuriot, S. Heyte, S. Paul, Guillaume Duflos and E. Heuson

Bio2Actives, 05-07/07, Quimper, France (2017)


4 - High-Throughput development of heterogeneous catalysts and processes for biomass valorisation

S. Paul, S. Heyte

Sichuan University, 09/06, Chengdu, China, (2017)


5 - REALCAT: A new high-throughput platform dedicated to the design of biorefineries catalysts

E. Heuson, S. Heyte, J. Thuriot, F. Dumeignil, S. Paul

Invited Lecture, 27/02, Pisa, Italy (2017)


6 - The REALCAT platform: high-throughput screening equipment dedicated to new enzymes discovery and process design for biomass valorization.

E. Heuson, A. Gimbernat, R. Froidevaux, J.-S. Girardon, S. Heyte, J. Thuriot, F. Dumeignil, S. Paul

Invited Lecture, 26/10-01/11, Nanning, China (2016)


7 - Valorisation of glycerol: Catalysts and processes

S. Paul, B. Katryniok, F. Dumeignil

UNICAT, 01/12, Université Fédérale de Rio de Janeiro, Rio De Janeiro, Brazil (2015)


8 - REALCAT: A new high-throughput platform dedicated to the design of biorefineries catalysts

S. Paul, S. Heyte, B. Katryniok, M. Araque Marin, F. Dumeignil

Catalysis Research Center, 22/06, Sapporo, Japan (2015)


9 - REALCAT: A new advanced high-throughput platform dedicated to the design of biorefineries catalysts

F. Dumeignil, S. Heyte, S. Paul

3rd Indo-French Bilateral Symposium on Catalysis for Sustainable And Environmental Chemistry, 30/10, Pune, India (2014)


10 - Culture medium optimization using high throughput approach in order to improve surfactin productivity by B. subtilis in a continuous process

L.F. Motta-Santos, F. Coutte, L. Tournier-Couturier, P. Dhulster, P. Jacques

10th ESBES and 6th IFIBiop scientific meetings 2014, 07-10/09, Lille, France (2014)


11 - Realcat: a new platform to bring catalysis to the lightspeed

S. Paul, S. Heyte, F. Dumeignil

NEXTLAB 2014, 02-04/04, Rueil-Malmaison, France (2014)


12 - High Throughput Experimentation for evaluation of cobalt and Iron Fischer-Tropsch Catalysts

V. Ordomsky, K. Cheng, M. Virginie, A. Khodakov

NEXTLAB 2014, 02-04/04, Rueil-Malmaison, France (2014)


13 - REALCAT: plate-forme technologique pour la conception de catalyseurs hybrides à haut débit pour les bioraffineries

P. Dhulster, P. Jacques, R. Froidevaux, S. Paul, S. Desset, F. Dumeignil

SFGP2013, 08-10/10, Lyon, France (2013)


14 - REALCAT: A new high-throughput platform dedicated to biorefineries catalysts design

S. Paul, S. Heyte, F. Dumeignil

4th International Environmental Best Practices Conference (EBP-IV), 08-12/09, Olsztyn, Poland (2013)


Affiches

1 - REALCAT: An Integrated and Advanced High-Throughput Platform for Catalysts Synthesis, Characterisation and Testing

S. Paul, S. Heyte, J. Thuriot-Roukos, F. Dumeignil

18th Nordic Symposium on Catalysis, 26-28/08, Copenhagen, Denmark, (2018).


2 - Selective oxidation of furfural and 5-methyl furfural under green conditions using supported gold nanoparticles

B. Reghizzi, F. Cavani, S. Paul, R. Wojcieszak

International Symposium on Relations between Homogeneous and Heterogeneous Catalysis, 22-25/07, Sydney, Australia (2018)


3 - Design of a multi-well plate for high-throughput characterization of heterogeneous catalysts by XRD, FT-IR, Raman, and XRF spectroscopy

J. Thuriot, S. Heyte, M. Bennis, E. Heuson, P. Roussel, F. Dumeignil, S. Paul

Europacat 13, 27-31/08, Firenze, Italy (2017)


4 - Alternatives to sulfites for shrimp preservation: - Standardized assay of 40 potential inhibitors of melanosis -

E. Zeyer, V. Phalip, C. Himber, C. Lebris, P. Dhulster, A. Brisabois, C. Flahaut, B. Cudennec, T. Grard, G. Duflos and E. Heuson

BioTrans 2017, 09-13/07, Budapest, Hungary (2017)


5 - Alternatives to sulfites for shrimp preservation: - Standardized assay of 40 potential inhibitors of melanosis -

E. Zeyer, V. Phalip, C. Himber, C. Lebris, P. Dhulster, A. Brisabois, C. Flahaut, B. Cudennec, T. Grard, G. Duflos and E. Heuson

Bio2Actives, 05-07/07, Quimper, France (2017)


6 - High-throughput screening of enzymatic cocktails obtained from the interaction of Zymoseptoria tritici with wheat straw

R. Raulo, E. Heuson, A. Siah, F. Krier, P. Halama, P. Reignault, V. Phalip, R. Froidevaux

SFR Condorcet, 08-09/06, Lille, France (2017)


7 - Advanced high throughput bio(chemical) technologies platform for biorefineries hybrid catalysts design

E. Heuson, A. Gimbernat, R. Vincent, S. Heyte, R. Froidevaux, S.Paul, P. Dhulster and F. Dumeignil

Exploring Lignocellulosic Biomass, 23-24/06, Reims, France (2016)


8 - Ethanol-to-propylene reaction catalyzed by ion-exchanged ZSM-5s

M. Ammoury, B. Katryniok, S. Heyte, G. Pomalaza, K. Shimizu, S. Paul, F. Dumeignil, M. Capron

FCCAT1, 23-27/05, Fréjus, France (2016)


9 - New trends in the production of green hydrocarbons from fatty acids via catalytic decarboxylation reactions

A. M. Kiméné, C. Durlin, O. Simon, R. Wojcieszak, S. Paul

FCCAT1, 23-27/05, Fréjus, France (2016)


10 - Realcat: A new powerful high-throughput platform dedicated to the design of biorefineries catalysts

S. Paul, F. Dumeignil, S. Heyte, M. Araque Marin

3rd International Symposium on Green Chemistry, 03-07/05, La Rochelle, France (2015)


11 - Accelerated Development Process in the First Asymmetric Hydrogenation of New 2-Substituted Quinoxalines Esters

A. M. Maj, S. Heyte, M. Araque-Marin, F. Dumeignil, S. Paul, I. Suisse, F. Agbossou-Niedercorn

19th Sigma-Aldrich Symposium, 10-11/12, DuinsePolders in Blankenberge, Belgium (2015)


12 - Highly efficient Fischer-Tropsch synthesis over Co catalysts on carbon containing inorganic supports

V. Subramanian, A. Khodakov, K. Cheng, S. Heyte, S. Paul, V. V. Ordomsky

Europacat 12, 30/08-04/09, Kazan, Russia (2015)


13 - REALCAT: A new high-throughput platform dedicated to the R&D in catalysis for biorefineries

S. Paul, S. Heyte, J. Thuriot Roukos, M. Araque Marina, F. Dumeignil

Europacat 12, 30/08-04/09, Kazan, Russia (2015)


14 - Realcat: une nouvelle plateforme de criblage haut-débit dédiée au développement de procédés catalytiques pour les bioraffineries

S. Paul, S. Heyte, J. Thuriot, M. Araque Marin, F. Dumeignil

Congrès de la Congrès de la Société Chimique SCF'15 « Chimie et transition énergétique », 04-09/07, Lille, France (2015)


15 - Catalytic Transformation of Ethanol into Propylene

M. Ammoury, B. Katryniok, S. Heyte, M. Araque-Marin, S. Paul, F. Dumeignil, M. Capron

Congrès de la Congrès de la Société Chimique de France SCF'15 « Chimie et transition énergétique », 04-09/07, Lille, France (2015)


16 - Catalysed Ethanol-to-Propene Conversion over FLOWRENCE® Apparatus

M. Ammoury, B. Katryniok, S. Heyte, M. Araque-Marin, S. Paul, F. Dumeignil, M. Capron

GECat 2015, 26-29/05, Obernai, France (2015)


17 - High-throughput study of glycerol catalytic dehydration to acrolein over ZrO2-SiO2-supported phosphotungstic acid

B. Katryniok, C. Garcà-Sancho, P. Maireles-Torres, F. Dumeignil, S. Paul

TOCAT-7, 01-06/06, Kyoto, Japon (2014)


Communications orales

1 - Catalytic Activation of CO2 towards Carboxylic Acids and Esters Mediated by Organometallic Precursors

K. Kunihiroa, S. Heyte, S. Paul, J.F Carpentiera, and E. Kirillov

GECOM-CONCOORD 2019, 19-24/06, Erquy, France (2019)


2 - Insight into the mechanism of base free furfural oxidation using Raman spectroscopy

J. Thuriot, R. Khadraoui, S. Paul, R. Wojcieszak

ISGC 2019, 13-17/05, La Rochelle, France (2019)


3 - Méthodes de criblage haut-de?bit en catalyse - Plateforme REALCAT

S. Paul

Journe?es des Jeunes Chercheurs en Ge?nie des Proce?de?s et Energe?tique 5e?me Edition France Wallonie, 20-21/11, Villeneuve D'Ascq, France (2018)


4 - A new two-step green process for 2,5-furandicarboxylic acid production from furfural, oxygen and carbon dioxide

S. Paul, R. Wojcieszak, F. Dumeignil, F. Santarelli, B. Rhegizzi, A. Roselli, F. Cavani, G. R. Dick, M. W. Kanan

TOCAT8, 5-10/08, Yokohama, Japan (2018)


5 - Pt-Pd/TiO2 catalysts for glucose hydrogenation: looking for a bimetallic synergy

A. Mazzi, A. da Silva, T. S. Rodrigues, S. Paul, P. H. C. Camargo, R. Wojcieszak

International Symposium on Relations between Homogeneous and Heterogeneous Catalysis, 22-25/07, Sydney, Australia (2018)


6 - Bimetallic Fe-Ni/SiO2 catalysts: preparation of Fe-Ni nanoparticles of controlled size and composition, and identification of the interplay between the two metals

D. Shi, Q. Yang, C. Peterson, A.-F. Lamic-Humblot, J.-S. Girardon, A. Constant-Griboval, A.-S. Mamede, M. Marinova, V. Briois, P. A. J. Bagot, R. Wojcieszak, S. Paul, E. Marceau

PREPA12, 12th International Symposium on the "Scientific Bases for the Preparation of Heterogeneous Catalysts", 8-12/07, Louvain-la-Neuve, Belgique (2018)


7 - Innovative high-throughput microplate approach for cell wall degrading enzyme production based on fungi and lignocellulosic raw biomass interaction

Roxane Raulo, E. Heuson, A. Siah, F. Krier, P. Halama, P. Reignault, V. Phalip, R. Froidevaux

Exploring Lignocellulosic Biomass, 26-29/06, Reims, France (2018)


8 - Advanced High-Throughput Technologies for Catalysts Design

S. Paul, S. Heyte, J. Thuriot-Roukos, F. Dumeignil

5th International School-Conference on Catalysis for Young Scientists “Catalyst Design: From Molecular to Industrial Level”, 20-23/06, Moscow, Russia (2018)


9 - Innovative high-throughput microplate approach for cell wall degrading enzyme production based on fungi and lignocellulosic raw biomass interaction

E. Heuson, Roxane Raulo, A. Siah, F. Krier, P. Halama, P. Reignault, V. Phalip, R. Froidevaux

CBSO, 22-25/05, Guidel Plage, France (2018)


10 - Influence de la formulation de catalyseurs bimétalliques Fe-Ni/SiO2 sur la conversion du furfural en alcool furfurylique

D. Shi, R. Wojcieszak, A.-S. Mamede, A.-F. Lamic-Humblot, S. Paul, E. Marceau

GECAT 2018, 22-25/05, Trégunc, France (2018)


11 - Kinetic Modeling of the Direct Amination of n-Octanol with Ammonia over a Ag- Co/Al2O3 catalyst

J. Ibanez, S. Paul, M. Araque-Marin and M. Pera-Titus

2nd International Conference on Catalysis and Chemical Engineering (CCE-2018), 19-21/02, Paris, France (2018)


12 - High-Throughput study of Ni- and Cu-based supported catalysts for low temperature hydrogenation of glucose to sorbitol

R. Wojcieszak, F. Ramos Neves, J. Sha, J. Thuriot, S. Heyte, A. Mazzi, L. Silvester, F. Dumeignil, M. Araque Marin, S. Paul

CATBIOR4, 11-15/12, Lyon, France (2017)


13 - Synthèse organocatalysée et caractérisation mécanique de polylactides étoilés à cœur saccharidique

A. Mebarki, A. Favrelle, S. Paul, F. Cazaux, P. Zinck, M. Brieu

JEPO’2017, 1-6/10, Gravelines, France (2017)


14 - The REALCAT platform: high-throughput screening equipment dedicated to biomass valorization.

E. Zeyer, B. Cudennec, C. Le Bris, T. Grard, C. Flahaut, B. Deracinois, P. Dhulster, R. Froidevaux, J. Thuriot, S. Heyte, S. Paul, Guillaume Duflos and E. Heuson

Bioingest, 11/09, Lille, France (2017)


15 - High-Throughput Development of a Catalytic Process for Glucose Hydrogenation to Sorbitol using the REALCAT platform

R. Wojcieszak, F. Ramos Neves, J. Sha, J. Thuriot, S. Heyte, A. Mazzi, L. Silvester, F. Dumeignil, M. Araque Marin, S. Paul

4th French-Chinese Symposium « Exploring New Challenges in Catalytic Science », 05/09, Lille, France (2017)


16 - One step sustainable synthesis of adipic acid

A. Mazzi, S. Paul, F. Cavani, R. Wojcieszak

Europacat 2017, 27-31/08, Firenze, Italy (2017)


17 - High-throughput screening of enzymatic cocktails obtained from the interaction of Zymoseptoria tritici with wheat straw

R. Raulo, E. Heuson, A. Siah, F. Krier, P. Halama, P. Reignault, V. Phalip, R. Froidevaux

2nd Symposium on Plant Biomass Conversion by Fungi, 28-29/08, Utrecht, The Netherlands (2017)


Brevets

1 - Module porte-échantillons destiné au traitement thermique de matériaux solides

S. Heyte, S. Paul, J. Faye

WO: 2019 008246 - 10/01/2019


2 - Procédé de production de 5-hydroxymethylfurfural à partir d'héxoses

A. Gimbernat, J.-S. Girardon, N. Lopes Ferreira, D. Damien, R. Froidevaux, P. Dhulster

n° de publication : 3 068 036

n° d'enregistrement national : 17 55668

Date de dépôt : 21/06/2017

Date de publication : 28/12/2018


3 - Production d'hydrocarbures linéaires par décarboxylation d'acides gras carboxyliques en présence d'un catalyseur bimétallique supporté

A. Mapembe Kimene, S. Paul, R. Wojcieszak

n° de publication : 3 066 193

n° d'enregistrement national : 17 54140

Date de dépôt : 11/05/2017

Date de publication : 16/11/2018


4 - Furoic acid preparation method

F. Santarelli, R. Wojcieszak, S. Paul, F. Dumeignil, F. Cavani

WO: 2017 158106 - 21/09/2017


5 - Use of molybdenum and vanadium mixed oxides as catalysts for the oxidation of unsaturated alcohols into insaturated carboxylic acids

S. Paul, F. Dumeignil, B. Katryniok, M. Araque Marin, T. Murayama, W. Ueda

WO: 2016 203283 - 22/12/2016


6 - Procédé de transformation sélective de polyols biosourcés en cétoses

M. Guehl, D. Delcroix, N. Lopes Ferreira, S. Desset, F. Dumeignil

n° de publication : 3 031 983

n° d'enregistrement national : 15 50532

Date de dépôt : 23/01/2015

Date de publication : 29/07/2016